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Capabilities

This page summarizes what the current user manual documents. It is not a promise that every combination of method, property, and backend is available. When a workflow has limits, use the linked workflow page or keyword page for the specific input contract.

Electronic Structure

Area Status
HF and DFT RHF, ROHF, and UHF references.
MP2 Energy-only standalone MP2 on RHF, UHF, and ROHF references, with spin-scaled variants.
TDHF/TDDFT Energy and gradient workflows for supported references.
SF-TDDFT and MRSF-TDDFT Multiconfigurational ground- and excited-state energies, gradients, NACME, SOC, and optimization workflows.
UMRSF-TDDFT Energy-only UHF-reference workflow.
MRSF-EKT IP/EA analysis with Dyson-like orbital data.

Properties

Property Status
Analytic gradients Available for the supported HF/DFT and response workflows.
HF/DFT Hessians Native analytic path for supported HF/DFT references.
Numerical Hessians Available through the Hessian workflow.
NACME MRSF-TDDFT state-coupling workflow.
SOC MRSF-TDDFT one-electron and mean-field two-electron SOC.
MRSF excited-state analysis NTOs, attachment/detachment densities, state-to-state transition densities, cube export, QCSchema export, FCIDUMP export, and external-code comparisons through oqp.interop.
Nonadiabatic MD (NAMD) Development preview in OpenQP PR #205, not OpenQP 1.2.0. Covers Tully surface hopping, SOC-NAMD, and ESPF QM/MM embedding. See SOC-NAMD-QMMM.
QM/MM Development preview in OpenQP PR #205, not OpenQP 1.2.0. Covers ESPF electrostatic embedding for single-point energies, ground-state MD, and nonadiabatic dynamics. See [qmmm].
Scalar relativistic correction Spin-free DKH correction through [scf] scal_rel=1 or 2.
PCM/ddX Energy-only reference-SCF path for RHF/ROHF.
NMR Nuclear magnetic shielding via [properties] scf_prop=nmr.
IR/Raman Frequency-analysis intensities from supported Hessian workflows.

Geometry and Paths

The native optimizer supports optimize, ts, meci, mecp, neb, irc, and mep; legacy tci inputs remain compatible. MECI includes the BaekA adaptive algorithm for two or more same-manifold states. Concise .oqp geometry drivers select the native engine automatically and do not expose a backend selector. Native TS supports model, numerical, or analytical initial Hessians and mode following. Native NEB supports endpoint alignment and relaxation, climbing images, maximum and RMS force convergence, and final multi-frame XYZ path output.

geomeTRIC and SciPy remain optional compatibility backends for traditional sectioned .inp files and the Python API. Native .oqp supports frozen-distance minimum searches; legacy geomeTRIC remains an escape hatch for advanced constraint types that the concise grammar does not yet support.

Upcoming or Limited Areas

  • Electrostatic embedding QM/MM is an active development direction. Nonadiabatic QM/MM dynamics currently supports whole-molecule QM regions only; covalent QM/MM boundaries (link atoms) in dynamics are not yet available.
  • PCM gradients, PCM optimizations, and state-specific excited-state PCM are not part of the first ddX energy path.
  • MP2 gradients, Hessians, RI/Laplace/local MP2 kernels, and periodic MP2 are not part of the documented standalone MP2 path.
  • UMRSF-TDDFT gradients and Hessians are not part of the documented production surface yet.